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Present work gives the general impression on carbon nanomaterials, including heterosubstituted, can be obtained pyrolytically. It is mostly focused on nanotubes and nanofibers, few layers nanoflakes and foams. The results of HRTEM, XPS, and thermal analysis of these materials are described to trace structural and chemical properties evolution of the materials under discussion. The examples of the application of them in catalysis and energy storage systems are given.