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The measurements of the inverse magnetoelectric (ME) effect in a two-layered FeSiBNbCu/ Pb(Zr,Ti)O3 (Finemet/PZT) sample were performed employing magnetooptical method. To observe the effect, magnetization curves of the amorphous Finemet ribbon were measured in the presence of the electric field applied to the PZT plate. It was revealed that the inverse ME effect has different signs at different orientations of the external magnetic field applied to the Finemet ribbon.