Magnetic resonance spectroscopy on the spin-frustrated magnets YBaCo3MO7 (M= Al, Fe)статья
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Дата последнего поиска статьи во внешних источниках: 15 февраля 2024 г.
Аннотация:We present experimental results of combined electron spin resonance (ESR) and nuclear magnetic resonance (NMR) measurements on single crystals of the Swedenborgite-type compounds YBaCo 3 M O 7 (M= Al, Fe). The magnetic lattice of these materials can be described as stacks of strongly geometrically frustrated kagome layers built up of Co 2+(S= 3/2) ions. Due to the Co-M site intermixing, there are M-type defects in the kagome planes as well as magnetic Co ions at the interplanar positions. Previous investigations revealed large antiferromagnetic (AFM) Curie-Weiss temperatures in both compounds. Yet no AFM long-range order but a spin glass behavior at low temperatures has been observed. Using Al 27 NMR as well as Co 2+ and Fe 3+ ESR spin probes that are sensitive to local magnetic properties at different crystallographic sites, we have identified two magnetic subsystems in both compounds