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Methane conversion in the presence of metal mesh electrodes and low-temperature discharge plasmaстатья
Статья опубликована в высокорейтинговом журнале
Информация о цитировании статьи получена из
Web of Science,
Scopus
Статья опубликована в журнале из списка Web of Science и/или Scopus
Дата последнего поиска статьи во внешних источниках: 5 декабря 2014 г.
- Авторы: Kobayashi K., Kulinich S.A., Ito T.
- Журнал: Journal of Applied Physics
- Том: 116
- Номер: 12
- Год издания: 2014
- Издательство: AIP Publishing
- Местоположение издательства: United States
- Первая страница: 123301
- Последняя страница: 123301
- DOI: 10.1063/1.4896359
- Аннотация: Methane gas conversion was studied in customized flow-type reactors with different dielectric barrier discharge generated in Ar-CH4-O2 gas mixtures. Different reactor geometries (with either volume or surface-type discharges) and different electrode materials were compared, and gas temperatures during methane conversion processes were evaluated. The discharge was generated by applying either a conventional sinusoid or nanosecond-pulsed voltage. The methane conversion rate was as high as 99% with the total gas flow rate of 15 sccm, while the temperatures did not exceed 450 K. No significant effect of electrode material (stainless steel, aluminum, or CuO coated copper) was found, confirming that the conversion temperatures were much lower than those required for activity of typical catalysts. The reactor geometry, flow rate, and oxygen amount could be used to govern both the methane conversion rate and the fractions of components in the final product.
- Добавил в систему: Кулинич Сергей Алексеевич
Прикрепленные файлы
| № | Имя | Описание | Имя файла | Размер | Добавлен |
|---|---|---|---|---|---|
| 1. | Полный текст | 069_JAP_2014.pdf | 1,1 МБ | 27 октября 2015 [skulinich] |